Al Lettieri is excellent in Godfather.
I don't know his name - but the actor who plays Sonny in Bronx Tale is very good.
Al Pacino in Carlito's Way and Scarface (though I suppose he isn't really a villain in Carlito's Way).
Samuel L Jackson - Pulp Fiction
Gary Oldman - True Romance
"My wife was weeping before she fell asleep, outside my window I saw my Caporegimes coming to the house and it is midnight. So, Consigliori of mine, I think you should tell your Don what everyone knows."
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